We are getting this error message when the Submit button on "Contact Us" page is clicked:
Request failed; Mailbox unavailable
you need to check with your hosting support that default emails are not working.
if they are not providing default email support then you can use the below extensions
https://github.com/magepal/magento2-gmail-smtp-app
OR
https://github.com/mageplaza/magento-2-smtp
both are good. you just need to install and configure with any email service provider.
kindly Accept as a Solution if this works for you and give Kudos